Tanuj Khattar
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Rapid initial state preparation for the quantum simulation of strongly correlated molecules and materials
Dominic Berry
Yu Tong
Alec White
Tae In Kim
Lin Lin
Seunghoon Lee
Garnet Chan
arXiv:2409.11748 (2024)
Preview abstract
Studies on quantum algorithms for ground state energy estimation often assume perfect ground state preparation; however, in reality the initial state will have imperfect overlap with the true ground state. Here we address that problem in two ways: by faster preparation of matrix product state (MPS) approximations, and more efficient filtering of the prepared state to find the ground state energy. We show how to achieve unitary synthesis with a Toffoli complexity about $7 \times$ lower than that in prior work, and use that to derive a more efficient MPS preparation method. For filtering we present two different approaches: sampling and binary search. For both we use the theory of window functions to avoid large phase errors and minimise the complexity. We find that the binary search approach provides better scaling with the overlap at the cost of a larger constant factor, such that it will be preferred for overlaps less than about 0.003. Finally, we estimate the total resources to perform ground state energy estimation of FeMoco and Iron cluster systems by estimating ground state overlap on an MPS initial state through extrapolation. With a modest bond dimension of 4000 we estimate a 0.96 overlap squared value producing total resources of $7.5 \times 10^{10}$ Toffoli gates; validating naive estimates where we assume perfect ground state overlap. These extrapolations allay practical concerns of exponential overlap decay in challenging-to-compute chemical systems.
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Expressing and Analyzing Quantum Algorithms with Qualtran
Charles Yuan
Anurudh Peduri
arXiv::2409.04643 (2024)
Preview abstract
Quantum computing's transition from theory to reality has spurred the need for novel software tools to manage the increasing complexity, sophistication, toil, and chance for error of quantum algorithm development. We present Qualtran, an open-source library for representing and analyzing quantum algorithms. Using carefully chosen abstractions and data structures, we can simulate and test algorithms, automatically generate information-rich diagrams, and tabulate resource requirements. Qualtran offers a \emph{standard library} of algorithmic building blocks that are essential for modern cost-minimizing compilations. Its capabilities are showcased through the re-analysis of key algorithms in Hamiltonian simulation, chemistry, and cryptography. The resulting architecture-independent resource counts can be forwarded to our implementation of cost models to estimate physical costs like wall-clock time and number of physical qubits assuming a surface-code architecture. Qualtran provides a foundation for explicit constructions and reproducible analysis, fostering greater collaboration within the quantum algorithm development community. We believe tools like Qualtran will accelerate progress in the field.
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Dynamics of magnetization at infinite temperature in a Heisenberg spin chain
Trond Andersen
Rhine Samajdar
Andre Petukhov
Jesse Hoke
Dmitry Abanin
ILYA Drozdov
Xiao Mi
Alexis Morvan
Charles Neill
Rajeev Acharya
Richard Ross Allen
Kyle Anderson
Markus Ansmann
Frank Arute
Kunal Arya
Juan Atalaya
Gina Bortoli
Alexandre Bourassa
Leon Brill
Michael Broughton
Bob Buckley
Tim Burger
Nicholas Bushnell
Juan Campero
Hung-Shen Chang
Jimmy Chen
Benjamin Chiaro
Desmond Chik
Josh Cogan
Roberto Collins
Paul Conner
William Courtney
Alex Crook
Ben Curtin
Agustin Di Paolo
Andrew Dunsworth
Clint Earle
Lara Faoro
Edward Farhi
Reza Fatemi
Vinicius Ferreira
Ebrahim Forati
Brooks Foxen
Gonzalo Garcia
Élie Genois
William Giang
Dar Gilboa
Raja Gosula
Alejo Grajales Dau
Steve Habegger
Michael Hamilton
Monica Hansen
Sean Harrington
Paula Heu
Gordon Hill
Markus Hoffmann
Trent Huang
Ashley Huff
Bill Huggins
Sergei Isakov
Justin Iveland
Cody Jones
Pavol Juhas
Marika Kieferova
Alexei Kitaev
Andrey Klots
Alexander Korotkov
Fedor Kostritsa
John Mark Kreikebaum
Dave Landhuis
Pavel Laptev
Kim Ming Lau
Lily Laws
Joonho Lee
Kenny Lee
Yuri Lensky
Alexander Lill
Wayne Liu
Salvatore Mandra
Orion Martin
Steven Martin
Seneca Meeks
Amanda Mieszala
Shirin Montazeri
Ramis Movassagh
Wojtek Mruczkiewicz
Ani Nersisyan
Michael Newman
JiunHow Ng
Murray Ich Nguyen
Tom O'Brien
Seun Omonije
Alex Opremcak
Rebecca Potter
Leonid Pryadko
David Rhodes
Charles Rocque
Negar Saei
Kannan Sankaragomathi
Henry Schurkus
Christopher Schuster
Mike Shearn
Aaron Shorter
Noah Shutty
Vladimir Shvarts
Vlad Sivak
Jindra Skruzny
Clarke Smith
Rolando Somma
George Sterling
Doug Strain
Marco Szalay
Doug Thor
Alfredo Torres
Guifre Vidal
Cheng Xing
Jamie Yao
Ping Yeh
Juhwan Yoo
Grayson Young
Yaxing Zhang
Ningfeng Zhu
Jeremy Hilton
Anthony Megrant
Yu Chen
Vadim Smelyanskiy
Vedika Khemani
Sarang Gopalakrishnan
Tomaž Prosen
Science, 384 (2024), pp. 48-53
Preview abstract
Understanding universal aspects of quantum dynamics is an unresolved problem in statistical mechanics. In particular, the spin dynamics of the one-dimensional Heisenberg model were conjectured as to belong to the Kardar-Parisi-Zhang (KPZ) universality class based on the scaling of the infinite-temperature spin-spin correlation function. In a chain of 46 superconducting qubits, we studied the probability distribution of the magnetization transferred across the chain’s center, P(M). The first two moments of P(M) show superdiffusive behavior, a hallmark of KPZ universality. However, the third and fourth moments ruled out the KPZ conjecture and allow for evaluating other theories. Our results highlight the importance of studying higher moments in determining dynamic universality classes and provide insights into universal behavior in quantum systems.
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Stable quantum-correlated many-body states through engineered dissipation
Xiao Mi
Alexios Michailidis
Sara Shabani
Jerome Lloyd
Rajeev Acharya
Igor Aleiner
Trond Andersen
Markus Ansmann
Frank Arute
Kunal Arya
Juan Atalaya
Gina Bortoli
Alexandre Bourassa
Leon Brill
Michael Broughton
Bob Buckley
Tim Burger
Nicholas Bushnell
Jimmy Chen
Benjamin Chiaro
Desmond Chik
Charina Chou
Josh Cogan
Roberto Collins
Paul Conner
William Courtney
Alex Crook
Ben Curtin
Alejo Grajales Dau
Dripto Debroy
Agustin Di Paolo
ILYA Drozdov
Andrew Dunsworth
Lara Faoro
Edward Farhi
Reza Fatemi
Vinicius Ferreira
Ebrahim Forati
Brooks Foxen
Élie Genois
William Giang
Dar Gilboa
Raja Gosula
Steve Habegger
Michael Hamilton
Monica Hansen
Sean Harrington
Paula Heu
Markus Hoffmann
Trent Huang
Ashley Huff
Bill Huggins
Sergei Isakov
Justin Iveland
Cody Jones
Pavol Juhas
Kostyantyn Kechedzhi
Marika Kieferova
Alexei Kitaev
Andrey Klots
Alexander Korotkov
Fedor Kostritsa
John Mark Kreikebaum
Dave Landhuis
Pavel Laptev
Kim Ming Lau
Lily Laws
Joonho Lee
Kenny Lee
Yuri Lensky
Alexander Lill
Wayne Liu
Orion Martin
Amanda Mieszala
Shirin Montazeri
Alexis Morvan
Ramis Movassagh
Wojtek Mruczkiewicz
Charles Neill
Ani Nersisyan
Michael Newman
JiunHow Ng
Murray Ich Nguyen
Tom O'Brien
Alex Opremcak
Andre Petukhov
Rebecca Potter
Leonid Pryadko
Charles Rocque
Negar Saei
Kannan Sankaragomathi
Henry Schurkus
Christopher Schuster
Mike Shearn
Aaron Shorter
Noah Shutty
Vladimir Shvarts
Jindra Skruzny
Clarke Smith
Rolando Somma
George Sterling
Doug Strain
Marco Szalay
Alfredo Torres
Guifre Vidal
Cheng Xing
Jamie Yao
Ping Yeh
Juhwan Yoo
Grayson Young
Yaxing Zhang
Ningfeng Zhu
Jeremy Hilton
Anthony Megrant
Yu Chen
Vadim Smelyanskiy
Dmitry Abanin
Science, 383 (2024), pp. 1332-1337
Preview abstract
Engineered dissipative reservoirs have the potential to steer many-body quantum systems toward correlated steady states useful for quantum simulation of high-temperature superconductivity or quantum magnetism. Using up to 49 superconducting qubits, we prepared low-energy states of the transverse-field Ising model through coupling to dissipative auxiliary qubits. In one dimension, we observed long-range quantum correlations and a ground-state fidelity of 0.86 for 18 qubits at the critical point. In two dimensions, we found mutual information that extends beyond nearest neighbors. Lastly, by coupling the system to auxiliaries emulating reservoirs with different chemical potentials, we explored transport in the quantum Heisenberg model. Our results establish engineered dissipation as a scalable alternative to unitary evolution for preparing entangled many-body states on noisy quantum processors.
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Quantum Computation of Stopping power for Inertial Fusion Target Design
Dominic Berry
Alina Kononov
Alec White
Joonho Lee
Andrew Baczewski
Proceedings of the National Academy of Sciences, 121 (2024), e2317772121
Preview abstract
Stopping power is the rate at which a material absorbs the kinetic energy of a charged particle passing through it - one of many properties needed over a wide range of thermodynamic conditions in modeling inertial fusion implosions. First-principles stopping calculations are classically challenging because they involve the dynamics of large electronic systems far from equilibrium, with accuracies that are particularly difficult to constrain and assess in the warm-dense conditions preceding ignition. Here, we describe a protocol for using a fault-tolerant quantum computer to calculate stopping power from a first-quantized representation of the electrons and projectile. Our approach builds upon the electronic structure block encodings of Su et al. [PRX Quantum 2, 040332 2021], adapting and optimizing those algorithms to estimate observables of interest from the non-Born-Oppenheimer dynamics of multiple particle species at finite temperature. We also work out the constant factors associated with a novel implementation of a high order Trotter approach to simulating a grid representation of these systems. Ultimately, we report logical qubit requirements and leading-order Toffoli costs for computing the stopping power of various projectile/target combinations relevant to interpreting and designing inertial fusion experiments. We estimate that scientifically interesting and classically intractable stopping power calculations can be quantum simulated with
roughly the same number of logical qubits and about one hundred times more Toffoli gates than is required for state-of-the-art quantum simulations of industrially relevant molecules such as FeMoCo or P450.
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Fault-Tolerant Quantum Simulation of Materials Using Bloch Orbitals
Dominic Berry
Alec White
Eugene DePrince III
Sabrina Sicolo
Michael Kuehn
Michael Kaicher
Joonho Lee
PRX Quantum, 4 (2023), pp. 040303
Preview abstract
The simulation of chemistry is among the most promising applications of quantum computing. However, most prior work exploring algorithms for block encoding, time evolving, and sampling in the eigenbasis of electronic structure Hamiltonians has either focused on modeling finite-sized systems, or has required a large number of plane-wave basis functions. In this work, we extend methods for quantum simulation with Bloch orbitals constructed from symmetry-adapted atom-centered orbitals so that one can model periodic ab initio Hamiltonians using only a modest number of basis functions. We focus on adapting existing algorithms based on combining qubitization with tensor factorizations of the Coulomb operator. Significant modifications of those algorithms are required to obtain an asymptotic speedup leveraging translational (or, more broadly, Abelian) symmetries. We implement block encodings using known tensor factorizations and a new Bloch orbital form of tensor hypercontraction. Finally, we estimate the resources required to deploy our algorithms to classically challenging model materials relevant to the chemistry of lithium nickel oxide battery cathodes within the surface code. We find that even with these improvements, the quantum runtime of these algorithms is on the order of thousands of days and further algorithmic improvements are required to make realistic quantum simulation of materials practical.
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Measurement-induced entanglement and teleportation on a noisy quantum processor
Jesse Hoke
Matteo Ippoliti
Dmitry Abanin
Rajeev Acharya
Trond Andersen
Markus Ansmann
Frank Arute
Kunal Arya
Juan Atalaya
Gina Bortoli
Alexandre Bourassa
Leon Brill
Michael Broughton
Bob Buckley
Tim Burger
Nicholas Bushnell
Jimmy Chen
Benjamin Chiaro
Desmond Chik
Josh Cogan
Roberto Collins
Paul Conner
William Courtney
Alex Crook
Ben Curtin
Alejo Grajales Dau
Agustin Di Paolo
ILYA Drozdov
Andrew Dunsworth
Daniel Eppens
Edward Farhi
Reza Fatemi
Vinicius Ferreira
Ebrahim Forati
Brooks Foxen
William Giang
Dar Gilboa
Raja Gosula
Steve Habegger
Michael Hamilton
Monica Hansen
Paula Heu
Markus Hoffmann
Trent Huang
Ashley Huff
Bill Huggins
Sergei Isakov
Justin Iveland
Cody Jones
Pavol Juhas
Kostyantyn Kechedzhi
Marika Kieferova
Alexei Kitaev
Andrey Klots
Alexander Korotkov
Fedor Kostritsa
John Mark Kreikebaum
Dave Landhuis
Pavel Laptev
Kim Ming Lau
Lily Laws
Joonho Lee
Kenny Lee
Yuri Lensky
Alexander Lill
Wayne Liu
Orion Martin
Amanda Mieszala
Shirin Montazeri
Alexis Morvan
Ramis Movassagh
Wojtek Mruczkiewicz
Charles Neill
Ani Nersisyan
Michael Newman
JiunHow Ng
Murray Ich Nguyen
Tom O'Brien
Seun Omonije
Alex Opremcak
Andre Petukhov
Rebecca Potter
Leonid Pryadko
Charles Rocque
Negar Saei
Kannan Sankaragomathi
Henry Schurkus
Christopher Schuster
Mike Shearn
Aaron Shorter
Noah Shutty
Vladimir Shvarts
Jindra Skruzny
Clarke Smith
Rolando Somma
George Sterling
Doug Strain
Marco Szalay
Alfredo Torres
Guifre Vidal
Cheng Xing
Jamie Yao
Ping Yeh
Juhwan Yoo
Grayson Young
Yaxing Zhang
Ningfeng Zhu
Jeremy Hilton
Anthony Megrant
Yu Chen
Vadim Smelyanskiy
Xiao Mi
Vedika Khemani
Nature, 622 (2023), 481–486
Preview abstract
Measurement has a special role in quantum theory: by collapsing the wavefunction, it can enable phenomena such as teleportation and thereby alter the ‘arrow of time’ that constrains unitary evolution. When integrated in many-body dynamics, measurements can lead to emergent patterns of quantum information in space–time that go beyond the established paradigms for characterizing phases, either in or out of equilibrium. For present-day noisy intermediate-scale quantum (NISQ) processors, the experimental realization of such physics can be problematic because of hardware limitations and the stochastic nature of quantum measurement. Here we address these experimental challenges and study measurement-induced quantum information phases on up to 70 superconducting qubits. By leveraging the interchangeability of space and time, we use a duality mapping to avoid mid-circuit measurement and access different manifestations of the underlying phases, from entanglement scaling to measurement-induced teleportation. We obtain finite-sized signatures of a phase transition with a decoding protocol that correlates the experimental measurement with classical simulation data. The phases display remarkably different sensitivity to noise, and we use this disparity to turn an inherent hardware limitation into a useful diagnostic. Our work demonstrates an approach to realizing measurement-induced physics at scales that are at the limits of current NISQ processors.
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Purification-Based Quantum Error Mitigation of Pair-Correlated Electron Simulations
Thomas E O'Brien
Gian-Luca R. Anselmetti
Fotios Gkritsis
Vincent Elfving
Stefano Polla
William J. Huggins
Oumarou Oumarou
Kostyantyn Kechedzhi
Dmitry Abanin
Rajeev Acharya
Igor Aleiner
Richard Ross Allen
Trond Ikdahl Andersen
Kyle Anderson
Markus Ansmann
Frank Carlton Arute
Kunal Arya
Juan Atalaya
Michael Blythe Broughton
Bob Benjamin Buckley
Alexandre Bourassa
Leon Brill
Tim Burger
Nicholas Bushnell
Jimmy Chen
Yu Chen
Benjamin Chiaro
Desmond Chun Fung Chik
Josh Godfrey Cogan
Roberto Collins
Paul Conner
William Courtney
Alex Crook
Ben Curtin
Ilya Drozdov
Andrew Dunsworth
Daniel Eppens
Lara Faoro
Edward Farhi
Reza Fatemi
Ebrahim Forati
Brooks Riley Foxen
William Giang
Dar Gilboa
Alejandro Grajales Dau
Steve Habegger
Michael C. Hamilton
Sean Harrington
Jeremy Patterson Hilton
Markus Rudolf Hoffmann
Trent Huang
Ashley Anne Huff
Sergei Isakov
Justin Thomas Iveland
Cody Jones
Pavol Juhas
Marika Kieferova
Andrey Klots
Alexander Korotkov
Fedor Kostritsa
John Mark Kreikebaum
Dave Landhuis
Pavel Laptev
Kim Ming Lau
Lily MeeKit Laws
Joonho Lee
Kenny Lee
Alexander T. Lill
Wayne Liu
Orion Martin
Trevor Johnathan Mccourt
Anthony Megrant
Xiao Mi
Masoud Mohseni
Shirin Montazeri
Alexis Morvan
Ramis Movassagh
Wojtek Mruczkiewicz
Charles Neill
Ani Nersisyan
Michael Newman
Jiun How Ng
Murray Nguyen
Alex Opremcak
Andre Gregory Petukhov
Rebecca Potter
Kannan Aryaperumal Sankaragomathi
Christopher Schuster
Mike Shearn
Aaron Shorter
Vladimir Shvarts
Jindra Skruzny
Vadim Smelyanskiy
Clarke Smith
Rolando Diego Somma
Doug Strain
Marco Szalay
Alfredo Torres
Guifre Vidal
Jamie Yao
Ping Yeh
Juhwan Yoo
Grayson Robert Young
Yaxing Zhang
Ningfeng Zhu
Christian Gogolin
Nature Physics (2023)
Preview abstract
An important measure of the development of quantum computing platforms has been the simulation of increasingly complex physical systems. Prior to fault-tolerant quantum computing, robust error mitigation strategies are necessary to continue this growth. Here, we study physical simulation within the seniority-zero electron pairing subspace, which affords both a computational stepping stone to a fully correlated model, and an opportunity to validate recently introduced ``purification-based'' error-mitigation strategies. We compare the performance of error mitigation based on doubling quantum resources in time (echo verification) or in space (virtual distillation), on up to 20 qubits of a superconducting qubit quantum processor. We observe a reduction of error by one to two orders of magnitude below less sophisticated techniques (e.g. post-selection); the gain from error mitigation is seen to increase with the system size. Employing these error mitigation strategies enables the implementation of the largest variational algorithm for a correlated chemistry system to-date. Extrapolating performance from these results allows us to estimate minimum requirements for a beyond-classical simulation of electronic structure. We find that, despite the impressive gains from purification-based error mitigation, significant hardware improvements will be required for classically intractable variational chemistry simulations.
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Noise-resilient Majorana Edge Modes on a Chain of Superconducting Qubits
Alejandro Grajales Dau
Alex Crook
Alex Opremcak
Alexa Rubinov
Alexander Korotkov
Alexandre Bourassa
Alexei Kitaev
Alexis Morvan
Andre Gregory Petukhov
Andrew Dunsworth
Andrey Klots
Anthony Megrant
Ashley Anne Huff
Benjamin Chiaro
Bernardo Meurer Costa
Bob Benjamin Buckley
Brooks Foxen
Charles Neill
Christopher Schuster
Cody Jones
Daniel Eppens
Dar Gilboa
Dave Landhuis
Dmitry Abanin
Doug Strain
Ebrahim Forati
Edward Farhi
Emily Mount
Fedor Kostritsa
Frank Carlton Arute
Guifre Vidal
Igor Aleiner
Jamie Yao
Jeremy Patterson Hilton
Joao Basso
John Mark Kreikebaum
Joonho Lee
Juan Atalaya
Juhwan Yoo
Justin Thomas Iveland
Kannan Aryaperumal Sankaragomathi
Kenny Lee
Kim Ming Lau
Kostyantyn Kechedzhi
Kunal Arya
Lara Faoro
Leon Brill
Marco Szalay
Markus Rudolf Hoffmann
Masoud Mohseni
Michael Blythe Broughton
Michael Newman
Michel Henri Devoret
Mike Shearn
Nicholas Bushnell
Orion Martin
Paul Conner
Pavel Laptev
Ping Yeh
Rajeev Acharya
Rebecca Potter
Reza Fatemi
Roberto Collins
Sergei Isakov
Shirin Montazeri
Steve Habegger
Thomas E O'Brien
Trent Huang
Trond Ikdahl Andersen
Vadim Smelyanskiy
Vladimir Shvarts
Wayne Liu
William Courtney
William Giang
William J. Huggins
Wojtek Mruczkiewicz
Xiao Mi
Yaxing Zhang
Yu Chen
Yuan Su
Zijun Chen
Science (2022) (to appear)
Preview abstract
Inherent symmetry of a quantum system may protect its otherwise fragile states. Leveraging such protection requires testing its robustness against uncontrolled environmental interactions. Using 47 superconducting qubits, we implement the kicked Ising model which exhibits Majorana edge modes (MEMs) protected by a $\mathbb{Z}_2$-symmetry. Remarkably, we find that any multi-qubit Pauli operator overlapping with the MEMs exhibits a uniform decay rate comparable to single-qubit relaxation rates, irrespective of its size or composition. This finding allows us to accurately reconstruct the exponentially localized spatial profiles of the MEMs. Spectroscopic measurements further indicate exponentially suppressed hybridization between the MEMs over larger system sizes, which manifests as a strong resilience against low-frequency noise. Our work elucidates the noise sensitivity of symmetry-protected edge modes in a solid-state environment.
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Realizing topologically ordered states on a quantum processor
Y.-J. Liu
A. Smith
C. Knapp
M. Newman
N. C. Jones
Z. Chen
X. Mi
A. Dunsworth
I. Aleiner
F. Arute
K. Arya
J. Atalaya
R. Barends
J. Basso
M. Broughton
B. B. Buckley
N. Bushnell
B. Chiaro
R. Collins
W. Courtney
A. R Derk
D. Eppens
L. Faoro
E. Farhi
B. Foxen
A. Greene
S. D. Harrington
J. Hilton
T. Huang
W. J. Huggins
S. V. Isakov
K. Kechedzhi
A. N. Korotkov
F. Kostritsa
D. Landhuis
P. Laptev
O. Martin
M. Mohseni
S. Montazeri
W. Mruczkiewicz
J. Mutus
C. Neill
T. E. O'Brien
A. Opremcak
B. Pato
A. Petukhov
V. Shvarts
D. Strain
M. Szalay
Z. Yao
P. Yeh
J. Yoo
A. Megrant
Y. Chen
V. Smelyanskiy
A. Kitaev
M. Knap
F. Pollmann
Science, 374 (2021), pp. 1237-1241
Preview abstract
The discovery of topological order has revolutionized the understanding of quantum matter in modern physics and provided the theoretical foundation for many quantum error correcting codes. Realizing topologically ordered states has proven to be extremely challenging in both condensed matter and synthetic quantum systems. Here, we prepare the ground state of the emblematic toric code Hamiltonian using an efficient quantum circuit on a superconducting quantum processor. We measure a topological entanglement entropy of Stopo ≈ −0.95 × ln 2 and simulate anyon interferometry to extract the braiding statistics of the emergent excitations. Furthermore, we investigate key aspects of the surface code, including logical state injection and the decay of the non-local order parameter. Our results illustrate the topological nature of these states and demonstrate their potential for implementing the surface code.
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